Remarkable adsorption performance for trace lead (II) by Fe/Zn 2D metal organic nanosheets modified with triethylamine
Abstract
Abstract
Fe/Zn metal organic nanosheet (B-FeZn) was prepared using 1,4-benzenedicarboxylic acid and triethylamine. B-FeZn showed a remarkable trace-level lead (II) (Pb
2+
) adsorption performance. The removal rates reached ≥ 98% within 60 min. After five adsorption/desorption cycles, the adsorption capacity of B-FeZn for Pb
2+
was decreased by 17.10%. Langmuir isothermal model and pseudo-second-order kinetic model were applied to define the purification process via the adsorption with high fitting degrees. The maximum adsorption capacity reached 215.90 mg·g
−1
. The prepared B-FeZn material exhibits a remarkable performance, with a fast adsorption rate and a prominent regeneration performance, in the adsorption for trace Pb
2+
, providing a novel Pb
2+
adsorbent with a bright future in the Pb
2+
removal in industrial production.
Graphical abstract
Keywords
- Regeneration,
- Wastewater treatment,
- Adsorbent,
- Metal cation,
- Nanosheet
References
- Shi et al. (2020) Cu/N doped lignin for highly selective efficient removal of As(v) from polluted water (pp. 147-154) https://doi.org/10.1016/j.ijbiomac.2020.06.016
- Kumari et al. (2022) Rapid analysis of trace sulphite ion using fluorescent carbon dots produced from single use plastic cups (pp. 101-112)
- Quyang et al. (2022) Polyaniline improves granulation and stability of aerobic granular sludge https://doi.org/10.1007/s42114-022-00450-1
- Jain et al. (2020) Surfactant-assisted cerium oxide and its catalytic activity towards Fenton process for non-degradable dye 3(3) (pp. 430-441) https://doi.org/10.1007/s42114-020-00159-z
- Moussa et al. (2021) The performance of activated carbon/NiFe2O4 magnetic composite to retain heavy metal ions from aqueous solution (pp. 135-145) https://doi.org/10.1016/j.cjche.2020.07.036
- Moradi et al. (2021) Synthesis of GO/HEMA, GO/HEMA/TiO2, and GO/Fe3O4/HEMA as novel nanocomposites and their dye removal ability 4(4) (pp. 1185-1204) https://doi.org/10.1007/s42114-021-00353-7
- Ali Baig et al. (2021) Facile fabrication of Zn-doped SnO2 nanoparticles for enhanced photocatalytic dye degradation performance under visible light exposure 4(1) (pp. 114-126) https://doi.org/10.1007/s42114-020-00195-9
- Li et al. (2022) N-Fe-Gd co-doped TiO2/g-C3N4 nanosheet hybrid composites with superior photocatalytic dye degradation https://doi.org/10.1007/s42114-42021-00326-w
- Babu et al. (2020) Enhanced photocatalytic degradation of cationic dyes under visible light irradiation by CuWO4-RGO nanocomposite 3(2) (pp. 205-212) https://doi.org/10.1007/s42114-020-00149-1
- Fallah et al. (2020) Use of graphene substrates for wastewater treatment of textile industries 3(2) (pp. 187-193) https://doi.org/10.1007/s42114-020-00146-4
- Jain et al. (2020) Zinc oxide nanoparticle incorporated on graphene oxide: an efficient and stable photocatalyst for water treatment through the Fenton process 3(2) (pp. 231-242) https://doi.org/10.1007/s42114-020-00153-5
- Danish et al. (2020) Photoelectrochemical and photocatalytic properties of Fe@ZnSQDs/TiO2 nanocomposites for degradation of different chromophoric organic pollutants in aqueous suspension 3(4) (pp. 570-582) https://doi.org/10.1007/s42114-020-00187-9
- Liu et al. (2020) Fabrication and investigation on Ag nanowires/TiO2 nanosheets/graphene hybrid nanocomposite and its water treatment performance 3(3) (pp. 402-414) https://doi.org/10.1007/s42114-020-00164-2
- Zhang et al. (2021) Microwave hydrothermally synthesized WO3/UiO-66 nanocomposites toward enhanced photocatalytic degradation of rhodamine B 4(4) (pp. 1330-1342) https://doi.org/10.1007/s42114-021-00346-6
- Cheng et al. (2022) Cyclodextrin modified graphene membrane for highly selective adsorption of organic dyes and copper (II) Ions https://doi.org/10.30919/es8d603
- Cheng et al. (2021) One-step microwave hydrothermal preparation of Cd/Zr-bimetallic metal–organic frameworks for enhanced photochemical properties 4(1) (pp. 150-161) https://doi.org/10.1007/s42114-020-00199-5
- Nag and Cummins (2022) Human health risk assessment of lead (Pb) through the environmental-food pathway https://doi.org/10.1016/j.scitotenv.2021.151168
- Guo et al. (2021) Synthesis and characterization of ZnNiCr-layered double hydroxides with high adsorption activities for Cr(VI) (pp. 819-829) https://doi.org/10.1007/s42114-021-00260-x
- Sun et al. (2021) Corncob-derived activated carbon for efficient adsorption dye in sewage (pp. 61-73)
- Li et al. (2021) Adsorption of xanthate from aqueous solution by multilayer graphene oxide: an experimental and molecular dynamics simulation study (pp. 725-732) https://doi.org/10.1007/s42114-021-00310-4
- Yuan et al. (2020) Nanocellulose-based composite materials for wastewater treatment and waste-oil remediation (pp. 41-52)
- Ahmadi et al. (2021) Core–shell activated carbon-ZIF-8 nanomaterials for the removal of tetracycline from polluted aqueous solution 4(4) (pp. 1384-1397) https://doi.org/10.1007/s42114-021-00357-3
- Kordjazi et al. (2020) Super-hydrophilic/oleophobic chitosan/acrylamide hydrogel: an efficient water/oil separation filter (pp. 167-175) https://doi.org/10.1007/s42114-020-00150-8
- Shi et al. (2020) Zwitterionic glycine modified Fe/Mg-layered double hydroxides for highly selective and efficient removal of oxyanions from polluted water (pp. 8-15) https://doi.org/10.1016/j.jmst.2019.12.034
- Cheng et al. (2021) Poly(sodium-p-styrenesulfonate)-grafted UiO-66 composite membranes boosting highly efficient molecular separation for environmental remediation (pp. 562-573) https://doi.org/10.1007/s42114-021-00253-w
- Si et al. (2022) Janus phenol–formaldehyde resin and periodic mesoporous organic silica nanoadsorbent for the removal of heavy metal ions and organic dyes from polluted water https://doi.org/10.1007/s42114-022-00446-x
- Zhang et al. (2021) Ionic liquid modification of metal-organic framework endows high selectivity for phosphoproteins adsorption (pp. 144-154) https://doi.org/10.1016/j.aca.2020.12.046
- Zhang et al. (2021) A facile method to achieve dopamine polymerization in MOFs pore structure for efficient and selective removal of trace lead (II) ions from drinking water https://doi.org/10.1016/j.jhazmat.2020.124917
- Li et al. (2021) Zn-based metal organic framework-covalent organic framework composites for trace lead extraction and fluorescence detection of TNP https://doi.org/10.1016/j.jhazmat.2020.125021
- Yin et al. (2021) Selective removal of As(V) from wastewater with high efficiency by glycine-modified Fe/Zn-layered double hydroxides (pp. 360-370) https://doi.org/10.1007/s42114-021-00214-3
- Li et al. (2021) Ultrathin 2D catalysts with N-coordinated single Co atom outside Co cluster for highly efficient Zn-air battery https://doi.org/10.1016/j.cej.2021.129719
- Nidamanuri et al. (2020) Graphene and graphene oxide-based membranes for gas separation (pp. 3-16)
- Gijare et al. (2021) Reduced graphene oxide based electrochemical nonenzymatic human serum glucose sensor (pp. 110-119)
- Magne et al. (2022) Graphene and its derivatives: understanding the main chemical and medicinal chemistry roles for biomedical applications https://doi.org/10.1007/s40097-021-00444-3
- Wu (2022) Tunable terahertz perfect absorber based on graphene-photonic crystal hetero-structure (pp. 87-192-192) https://doi.org/10.30919/es8d498
- Cheng et al. (2021) Ultrathin flexible poly(vinylidene fluoride)/MXene/silver nanowire film with outstanding specific EMI shielding and high heat dissipation (pp. 502-513)
- Guo et al. (2021) Electrostatic self-assembled NiFe2O4/Ti3C2Tx MXene nanocomposites for efficient electromagnetic wave absorption at ultralow loading level (pp. 602-613) https://doi.org/10.1007/s42114-021-00279-0
- Wang et al. (2022) Electromagnetic interference shielding enhancement of poly(lactic acid)-based carbonaceous nanocomposites by poly(ethylene oxide)-assisted segregated structure: a comparative study of carbon nanotubes and graphene nanoplatelets https://doi.org/10.1007/s42114-021-00320-2
- Liu et al. (2021) Near-field radiative heat transfer via coupling graphene plasmons with different phonon polaritons in the reststrahlen bands https://doi.org/10.30919/es8d529
- Zhang et al. (2021) Constructing dual thermal conductive networks in electrospun polyimide membranes with highly thermally conductivity but electrical insulation properties (pp. 1102-1112) https://doi.org/10.1007/s42114-021-00335-9
- Gao et al. (2021) Flexible multilayered MXene/thermoplastic polyurethane films with excellent electromagnetic interference shielding, thermal conductivity, and management performances (pp. 274-285) https://doi.org/10.1007/s42114-021-00221-4
- Liu and Mao (2021) Graphene oxide-based nanomaterials for uranium adsorptive uptake (pp. 3-22)
- Lin et al. (2021) High-yield exfoliation of 2D semiconductor monolayers and reassembly of organic/inorganic artificial superlattices 7(7) (pp. 1887-1902) https://doi.org/10.1016/j.chempr.2021.03.022
- Kumar et al. (2021) MXenes: Emerging 2D materials for hydrogen storage https://doi.org/10.1016/j.nanoen.2021.105989
- Wang et al. (2020) Significantly enhanced Ultrathin NiCo-based MOF nanosheet electrodes hybrided with Ti3C2Tx MXene for high performance asymmetric supercapacitor (pp. 50-59)
- Pu et al. (2021) N-doped MXene derived from chitosan for the highly effective electrochemical properties as supercapacitor https://doi.org/10.1007/s42114-42021-00371-42115
- Wei et al. (2021) Fabrication of ternary MXene/MnO2/polyaniline nanostructure with good electrochemical performances (pp. 1082-1091) https://doi.org/10.1007/s42114-021-00323-z
- Budumuru and Satya Anuradha (2021) Electromagnetic shielding and mechanical properties of AL6061 metal matrix composite at X-band for oblique incidence (pp. 1113-1121) https://doi.org/10.1007/s42114-021-00338-6
- Hui et al. (2021) Reduced graphene oxide/nanocellulose/amino-multiwalled carbon nanotubes nanocomposite aerogel for excellent oil adsorption (pp. 38-44)
- Han et al. (2022) Flexible ethylene-vinyl acetate copolymer/fluorographene composite films with excellent thermal conductive and electrical insulation properties for thermal management (pp. 53-64)
- Yu et al. (2021) Effects of functional additives on structure and properties of polycarbonate-based composites filled with hybrid chopped carbon fiber/graphene nanoplatelet fillers (pp. 66-76)
- Cao et al. (2021) High strength, flexible, and conductive graphene/polypropylene fiber paper fabricated via papermaking process https://doi.org/10.1007/s42114-42021-00374-42112
- Xia et al. (2021) Superior wear resistance of epoxy composite with highly dispersed graphene spheres https://doi.org/10.1007/s42114-42021-00259-42114
- Bustero et al. (2020) Free-standing graphene films embedded in epoxy resin with enhanced thermal properties 3(1) (pp. 31-40) https://doi.org/10.1007/s42114-020-00136-6
- Wang et al. (2020) Hyperelastic magnetic reduced graphene oxide three-dimensional framework with superb oil and organic solvent adsorption capability 3(4) (pp. 473-484) https://doi.org/10.1007/s42114-020-00191-z
- Feng et al. (2020) Self-assembling 2D/2D (MXene/LDH) materials achieve ultra-high adsorption of heavy metals Ni2+ through terminal group modification https://doi.org/10.1016/j.seppur.2020.117525
- Han et al. (2018) Nickel metal-organic framework monolayers for photoreduction of diluted CO2: Metal-node-dependent activity and selectivity 57(51) (pp. 16811-16815) https://doi.org/10.1002/anie.201811545
- Chen et al. (2021) Fabrication of a novel Co/Ni-MOFs@BiOI composite with boosting photocatalytic degradation of methylene blue under visible light 9(5) https://doi.org/10.1016/j.jece.2021.106194
- Shi et al. (2021) Strong selectivity and high capacity in the adsorption of As (V) from wastewater by glycine-modified Fe/Cu-layered double hydroxides https://doi.org/10.1016/j.jallcom.2021.158956
- Shi et al. (2021) Preparation of Mg, N-co-doped lignin adsorbents for enhanced selectivity and high adsorption capacity of As (V) from wastewater (pp. 206-213) https://doi.org/10.1016/j.partic.2021.03.014
- Kong et al. (2020) Enhanced removal of vanadium(V) from groundwater by layered double hydroxide-supported nanoscale zerovalent iron https://doi.org/10.1016/j.jhazmat.2020.122392
- Xue et al. (2022) Amorphous Mn-La oxides immobilized on carbon sphere for efficient removal of As(V), Cd(II), and Pb(II): Co-adsorption and roles of Mn species https://doi.org/10.1016/j.cej.2021.132262
- Threepanich and Praipipat (2021) Powdered and beaded lemon peels-doped iron (III) oxide-hydroxide materials for lead removal applications: Synthesis, characterizations, and lead adsorption studies 9(5) https://doi.org/10.1016/j.jece.2021.106007
- Tang et al. (2021) Phenylthiosemicarbazide-functionalized UiO-66-NH2 as highly efficient adsorbent for the selective removal of lead from aqueous solutions https://doi.org/10.1016/j.jhazmat.2021.125278
- Du et al. (2017) Highly efficient removal of Pb2+ by a polyoxomolybdate-based organic-inorganic hybrid material {(4-Hap)4[Mo8O26]} 5(2) (pp. 1866-1873) https://doi.org/10.1016/j.jece.2017.03.028
- Song et al. (2018) The selectively fluorescent sensing detection and adsorptive removal of Pb2+ with a stable [δ-Mo8O26]-based hybrid (pp. 598-604) https://doi.org/10.1016/j.jcis.2018.08.029
- Zhong et al. (2021) Design and syntheses of functionalized copper-based MOFs and its adsorption behavior for Pb(II) https://doi.org/10.1016/j.cclet.2021.1007.1040
- Yang et al. (2022) Functionalized dual modification of covalent organic framework for efficient and rapid trace heavy metals removal from drinking water https://doi.org/10.1016/j.chemosphere.2021.133215
- Morcos et al. (2021) High performance functionalized UiO metal organic frameworks for the efficient and selective adsorption of Pb (II) ions in concentrated multi-ion systems 9(3) https://doi.org/10.1016/j.jece.2021.105191
- Hong et al. (2022) Highly efficient removal of trace lead (II) from wastewater by 1,4-dicarboxybenzene modified Fe/Co metal organic nanosheets (pp. 212-218) https://doi.org/10.1016/j.jmst.2021.05.021
- Jing et al. (2022) Improving thermal conductivity of polyethylene/polypropylene by styrene-ethylene-propylene-styrene wrapping hexagonal boron nitride at the phase interface https://doi.org/10.1007/s42114-022-00438-x
- Wang et al. (2022) Broadband radar-absorbing performance of square-hole structure (pp. 525-535) https://doi.org/10.1007/s42114-021-00376-0
- Xin et al. (2021) Ultrahigh specific strength in a magnesium alloy strengthened by spinodal decomposition https://doi.org/10.1126/sciadv.abf3039
- Zhang et al. (2021) Correlation of C/C preform density and microstructure and mechanical properties of C/C-ZrC-based ultra-high-temperature ceramic matrix composites (pp. 743-750) https://doi.org/10.1007/s42114-021-00295-0
- Luo et al. (2021) Study on broadband microwave absorbing performance of gradient porous structure (pp. 591-601) https://doi.org/10.1007/s42114-021-00275-4
- Shao et al. (2021) Study on favorable comprehensive properties of superhydrophobic coating fabricated by polytetrafluoroethylene doped with graphene (pp. 521-533) https://doi.org/10.1007/s42114-021-00243-y
- Chen et al. (2021) Reinforced AZ91D magnesium alloy with thixomolding process facilitated dispersion of graphene nanoplatelets and enhanced interfacial interactions https://doi.org/10.1016/j.msea.2021.140793
- Zhao et al. (2019) Phase-field simulation for the evolution of solid/liquid interface front in directional solidification process
- Song et al. (2021) Waterborne polyurethane/3-amino-polyhedral oligomeric silsesquioxane (NH2-POSS) nanocomposites with enhanced properties (pp. 629-638) https://doi.org/10.1007/s42114-021-00285-2
- Chen et al. (2021) Three-dimensional phase-field simulations of the influence of diffusion interface width on dendritic growth of Fe-0.5 wt.%C alloy (pp. 371-378) https://doi.org/10.1007/s42114-021-00215-2
- Zhao et al. (2022) Fabrication of magnesium-coated graphene and its effect on the microstructure of reinforced AZ91 magnesium-matrix composites (pp. 504-512) https://doi.org/10.1007/s42114-021-00336-8
- Liu et al. (2020) Impact of lithium salts on the combustion characteristics of electrolyte under diverse pressures https://doi.org/10.3390/en13205373
- Lai et al. (2022) Aqueous flexible all-solid-state NiCo-Zn batteries with high capacity based on advanced ion-buffering reservoirs of NiCo2O4 https://doi.org/10.1007/s42114-021-00375-1
- Xu et al. (2022) Enhancement of catalytic combustion and thermolysis for treating polyethylene plastic waste https://doi.org/10.1007/s42114-021-00317-x
- Tan et al. (2022) Long-life and dendrite-free zinc metal anode enabled by a flexible, green and self-assembled zincophilic biomass engineered MXene based interface https://doi.org/10.1016/j.cej.2021.134277
- Liu et al. (2020) Phase change materials application in battery thermal management system: A review https://doi.org/10.3390/ma13204622
- Yu et al. (2022) Effect of pressure on anisotropy in elasticity, sound velocity, and thermal conductivity of vanadium borides https://doi.org/10.1007/s42114-021-00403-0
- Liu et al. (2021) Experimental thermal hazard investigation of pressure and EC/PC/EMC mass ratio on electrolyte 14(9) https://doi.org/10.3390/en14092511
- Zhao et al. (2022) Three-dimensional printing of the copper sulfate hybrid composites for supercapacitor electrodes with ultra-high areal and volumetric capacitances https://doi.org/10.1007/s42114-022-00430-5
- Shen et al. (2021) Nanoscale niobium oxides anode for electrochemical lithium and sodium storage: a review of recent improvements (pp. 33-68) https://doi.org/10.1007/s40097-020-00367-5
- Liu et al. (2021) High ion selectivity aquivion-based hybrid membranes for all vanadium redox flow battery (pp. 451-458) https://doi.org/10.1007/s42114-021-00261-w
10.1007/s40097-022-00495-0