10.1007/s40097-022-00495-0

Remarkable adsorption performance for trace lead (II) by Fe/Zn 2D metal organic nanosheets modified with triethylamine

  • Junhua Li1,
  • Kunqi Liu2,
  • Mohamed M. Ibrahim3,
  • Xueyi Zhang2,
  • Gaber A. M. Mersal3,
  • Junmao Hong1,
  • Lingshu Gao2,
  • Xiaofeng Shi4,
  • Tao Ding5,
  • Vignesh Murugadoss5,
  • Suying Wei6,
  • Mina Huang5,
  • Zhanhu Guo*5,
  1. School of Chemical Engineering and Technology, North University of China, Taiyuan, CN
  2. School of Environment and Safety Engineering, North University of China, Taiyuan, CN
  3. Department of Chemistry, College of Science, Taif University, Taif, 21944, SA
  4. School of Chemical Engineering and Technology, North University of China, Taiyuan, CN School of Environment and Safety Engineering, North University of China, Taiyuan, CN
  5. Integrated Composites Laboratory (ICL), Department of Chemical and Bimolecular Engineering, University of Tennessee, Knoxville, TN, 37996, US
  6. Department of Chemistry and Biochemistry, Lamar University, Beaumont, TX, 77710, US

Published in Issue 18-05-2022

How to Cite

Li, J., Liu, K., Ibrahim, M. M., Zhang, X., Mersal, G. A. M., Hong, J., Gao, L., Shi, X., Ding, T., Murugadoss, V., Wei, S., Huang, M., & Guo, Z. (2022). Remarkable adsorption performance for trace lead (II) by Fe/Zn 2D metal organic nanosheets modified with triethylamine. Journal of Nanostructure in Chemistry, 12(4 (August 2022). https://doi.org/10.1007/s40097-022-00495-0
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Abstract

Abstract Fe/Zn metal organic nanosheet (B-FeZn) was prepared using 1,4-benzenedicarboxylic acid and triethylamine. B-FeZn showed a remarkable trace-level lead (II) (Pb 2+ ) adsorption performance. The removal rates reached ≥ 98% within 60 min. After five adsorption/desorption cycles, the adsorption capacity of B-FeZn for Pb 2+ was decreased by 17.10%. Langmuir isothermal model and pseudo-second-order kinetic model were applied to define the purification process via the adsorption with high fitting degrees. The maximum adsorption capacity reached 215.90 mg·g −1 . The prepared B-FeZn material exhibits a remarkable performance, with a fast adsorption rate and a prominent regeneration performance, in the adsorption for trace Pb 2+ , providing a novel Pb 2+ adsorbent with a bright future in the Pb 2+ removal in industrial production. Graphical abstract

Keywords

  • Regeneration,
  • Wastewater treatment,
  • Adsorbent,
  • Metal cation,
  • Nanosheet

References

  1. Shi et al. (2020) Cu/N doped lignin for highly selective efficient removal of As(v) from polluted water (pp. 147-154) https://doi.org/10.1016/j.ijbiomac.2020.06.016
  2. Kumari et al. (2022) Rapid analysis of trace sulphite ion using fluorescent carbon dots produced from single use plastic cups (pp. 101-112)
  3. Quyang et al. (2022) Polyaniline improves granulation and stability of aerobic granular sludge https://doi.org/10.1007/s42114-022-00450-1
  4. Jain et al. (2020) Surfactant-assisted cerium oxide and its catalytic activity towards Fenton process for non-degradable dye 3(3) (pp. 430-441) https://doi.org/10.1007/s42114-020-00159-z
  5. Moussa et al. (2021) The performance of activated carbon/NiFe2O4 magnetic composite to retain heavy metal ions from aqueous solution (pp. 135-145) https://doi.org/10.1016/j.cjche.2020.07.036
  6. Moradi et al. (2021) Synthesis of GO/HEMA, GO/HEMA/TiO2, and GO/Fe3O4/HEMA as novel nanocomposites and their dye removal ability 4(4) (pp. 1185-1204) https://doi.org/10.1007/s42114-021-00353-7
  7. Ali Baig et al. (2021) Facile fabrication of Zn-doped SnO2 nanoparticles for enhanced photocatalytic dye degradation performance under visible light exposure 4(1) (pp. 114-126) https://doi.org/10.1007/s42114-020-00195-9
  8. Li et al. (2022) N-Fe-Gd co-doped TiO2/g-C3N4 nanosheet hybrid composites with superior photocatalytic dye degradation https://doi.org/10.1007/s42114-42021-00326-w
  9. Babu et al. (2020) Enhanced photocatalytic degradation of cationic dyes under visible light irradiation by CuWO4-RGO nanocomposite 3(2) (pp. 205-212) https://doi.org/10.1007/s42114-020-00149-1
  10. Fallah et al. (2020) Use of graphene substrates for wastewater treatment of textile industries 3(2) (pp. 187-193) https://doi.org/10.1007/s42114-020-00146-4
  11. Jain et al. (2020) Zinc oxide nanoparticle incorporated on graphene oxide: an efficient and stable photocatalyst for water treatment through the Fenton process 3(2) (pp. 231-242) https://doi.org/10.1007/s42114-020-00153-5
  12. Danish et al. (2020) Photoelectrochemical and photocatalytic properties of Fe@ZnSQDs/TiO2 nanocomposites for degradation of different chromophoric organic pollutants in aqueous suspension 3(4) (pp. 570-582) https://doi.org/10.1007/s42114-020-00187-9
  13. Liu et al. (2020) Fabrication and investigation on Ag nanowires/TiO2 nanosheets/graphene hybrid nanocomposite and its water treatment performance 3(3) (pp. 402-414) https://doi.org/10.1007/s42114-020-00164-2
  14. Zhang et al. (2021) Microwave hydrothermally synthesized WO3/UiO-66 nanocomposites toward enhanced photocatalytic degradation of rhodamine B 4(4) (pp. 1330-1342) https://doi.org/10.1007/s42114-021-00346-6
  15. Cheng et al. (2022) Cyclodextrin modified graphene membrane for highly selective adsorption of organic dyes and copper (II) Ions https://doi.org/10.30919/es8d603
  16. Cheng et al. (2021) One-step microwave hydrothermal preparation of Cd/Zr-bimetallic metal–organic frameworks for enhanced photochemical properties 4(1) (pp. 150-161) https://doi.org/10.1007/s42114-020-00199-5
  17. Nag and Cummins (2022) Human health risk assessment of lead (Pb) through the environmental-food pathway https://doi.org/10.1016/j.scitotenv.2021.151168
  18. Guo et al. (2021) Synthesis and characterization of ZnNiCr-layered double hydroxides with high adsorption activities for Cr(VI) (pp. 819-829) https://doi.org/10.1007/s42114-021-00260-x
  19. Sun et al. (2021) Corncob-derived activated carbon for efficient adsorption dye in sewage (pp. 61-73)
  20. Li et al. (2021) Adsorption of xanthate from aqueous solution by multilayer graphene oxide: an experimental and molecular dynamics simulation study (pp. 725-732) https://doi.org/10.1007/s42114-021-00310-4
  21. Yuan et al. (2020) Nanocellulose-based composite materials for wastewater treatment and waste-oil remediation (pp. 41-52)
  22. Ahmadi et al. (2021) Core–shell activated carbon-ZIF-8 nanomaterials for the removal of tetracycline from polluted aqueous solution 4(4) (pp. 1384-1397) https://doi.org/10.1007/s42114-021-00357-3
  23. Kordjazi et al. (2020) Super-hydrophilic/oleophobic chitosan/acrylamide hydrogel: an efficient water/oil separation filter (pp. 167-175) https://doi.org/10.1007/s42114-020-00150-8
  24. Shi et al. (2020) Zwitterionic glycine modified Fe/Mg-layered double hydroxides for highly selective and efficient removal of oxyanions from polluted water (pp. 8-15) https://doi.org/10.1016/j.jmst.2019.12.034
  25. Cheng et al. (2021) Poly(sodium-p-styrenesulfonate)-grafted UiO-66 composite membranes boosting highly efficient molecular separation for environmental remediation (pp. 562-573) https://doi.org/10.1007/s42114-021-00253-w
  26. Si et al. (2022) Janus phenol–formaldehyde resin and periodic mesoporous organic silica nanoadsorbent for the removal of heavy metal ions and organic dyes from polluted water https://doi.org/10.1007/s42114-022-00446-x
  27. Zhang et al. (2021) Ionic liquid modification of metal-organic framework endows high selectivity for phosphoproteins adsorption (pp. 144-154) https://doi.org/10.1016/j.aca.2020.12.046
  28. Zhang et al. (2021) A facile method to achieve dopamine polymerization in MOFs pore structure for efficient and selective removal of trace lead (II) ions from drinking water https://doi.org/10.1016/j.jhazmat.2020.124917
  29. Li et al. (2021) Zn-based metal organic framework-covalent organic framework composites for trace lead extraction and fluorescence detection of TNP https://doi.org/10.1016/j.jhazmat.2020.125021
  30. Yin et al. (2021) Selective removal of As(V) from wastewater with high efficiency by glycine-modified Fe/Zn-layered double hydroxides (pp. 360-370) https://doi.org/10.1007/s42114-021-00214-3
  31. Li et al. (2021) Ultrathin 2D catalysts with N-coordinated single Co atom outside Co cluster for highly efficient Zn-air battery https://doi.org/10.1016/j.cej.2021.129719
  32. Nidamanuri et al. (2020) Graphene and graphene oxide-based membranes for gas separation (pp. 3-16)
  33. Gijare et al. (2021) Reduced graphene oxide based electrochemical nonenzymatic human serum glucose sensor (pp. 110-119)
  34. Magne et al. (2022) Graphene and its derivatives: understanding the main chemical and medicinal chemistry roles for biomedical applications https://doi.org/10.1007/s40097-021-00444-3
  35. Wu (2022) Tunable terahertz perfect absorber based on graphene-photonic crystal hetero-structure (pp. 87-192-192) https://doi.org/10.30919/es8d498
  36. Cheng et al. (2021) Ultrathin flexible poly(vinylidene fluoride)/MXene/silver nanowire film with outstanding specific EMI shielding and high heat dissipation (pp. 502-513)
  37. Guo et al. (2021) Electrostatic self-assembled NiFe2O4/Ti3C2Tx MXene nanocomposites for efficient electromagnetic wave absorption at ultralow loading level (pp. 602-613) https://doi.org/10.1007/s42114-021-00279-0
  38. Wang et al. (2022) Electromagnetic interference shielding enhancement of poly(lactic acid)-based carbonaceous nanocomposites by poly(ethylene oxide)-assisted segregated structure: a comparative study of carbon nanotubes and graphene nanoplatelets https://doi.org/10.1007/s42114-021-00320-2
  39. Liu et al. (2021) Near-field radiative heat transfer via coupling graphene plasmons with different phonon polaritons in the reststrahlen bands https://doi.org/10.30919/es8d529
  40. Zhang et al. (2021) Constructing dual thermal conductive networks in electrospun polyimide membranes with highly thermally conductivity but electrical insulation properties (pp. 1102-1112) https://doi.org/10.1007/s42114-021-00335-9
  41. Gao et al. (2021) Flexible multilayered MXene/thermoplastic polyurethane films with excellent electromagnetic interference shielding, thermal conductivity, and management performances (pp. 274-285) https://doi.org/10.1007/s42114-021-00221-4
  42. Liu and Mao (2021) Graphene oxide-based nanomaterials for uranium adsorptive uptake (pp. 3-22)
  43. Lin et al. (2021) High-yield exfoliation of 2D semiconductor monolayers and reassembly of organic/inorganic artificial superlattices 7(7) (pp. 1887-1902) https://doi.org/10.1016/j.chempr.2021.03.022
  44. Kumar et al. (2021) MXenes: Emerging 2D materials for hydrogen storage https://doi.org/10.1016/j.nanoen.2021.105989
  45. Wang et al. (2020) Significantly enhanced Ultrathin NiCo-based MOF nanosheet electrodes hybrided with Ti3C2Tx MXene for high performance asymmetric supercapacitor (pp. 50-59)
  46. Pu et al. (2021) N-doped MXene derived from chitosan for the highly effective electrochemical properties as supercapacitor https://doi.org/10.1007/s42114-42021-00371-42115
  47. Wei et al. (2021) Fabrication of ternary MXene/MnO2/polyaniline nanostructure with good electrochemical performances (pp. 1082-1091) https://doi.org/10.1007/s42114-021-00323-z
  48. Budumuru and Satya Anuradha (2021) Electromagnetic shielding and mechanical properties of AL6061 metal matrix composite at X-band for oblique incidence (pp. 1113-1121) https://doi.org/10.1007/s42114-021-00338-6
  49. Hui et al. (2021) Reduced graphene oxide/nanocellulose/amino-multiwalled carbon nanotubes nanocomposite aerogel for excellent oil adsorption (pp. 38-44)
  50. Han et al. (2022) Flexible ethylene-vinyl acetate copolymer/fluorographene composite films with excellent thermal conductive and electrical insulation properties for thermal management (pp. 53-64)
  51. Yu et al. (2021) Effects of functional additives on structure and properties of polycarbonate-based composites filled with hybrid chopped carbon fiber/graphene nanoplatelet fillers (pp. 66-76)
  52. Cao et al. (2021) High strength, flexible, and conductive graphene/polypropylene fiber paper fabricated via papermaking process https://doi.org/10.1007/s42114-42021-00374-42112
  53. Xia et al. (2021) Superior wear resistance of epoxy composite with highly dispersed graphene spheres https://doi.org/10.1007/s42114-42021-00259-42114
  54. Bustero et al. (2020) Free-standing graphene films embedded in epoxy resin with enhanced thermal properties 3(1) (pp. 31-40) https://doi.org/10.1007/s42114-020-00136-6
  55. Wang et al. (2020) Hyperelastic magnetic reduced graphene oxide three-dimensional framework with superb oil and organic solvent adsorption capability 3(4) (pp. 473-484) https://doi.org/10.1007/s42114-020-00191-z
  56. Feng et al. (2020) Self-assembling 2D/2D (MXene/LDH) materials achieve ultra-high adsorption of heavy metals Ni2+ through terminal group modification https://doi.org/10.1016/j.seppur.2020.117525
  57. Han et al. (2018) Nickel metal-organic framework monolayers for photoreduction of diluted CO2: Metal-node-dependent activity and selectivity 57(51) (pp. 16811-16815) https://doi.org/10.1002/anie.201811545
  58. Chen et al. (2021) Fabrication of a novel Co/Ni-MOFs@BiOI composite with boosting photocatalytic degradation of methylene blue under visible light 9(5) https://doi.org/10.1016/j.jece.2021.106194
  59. Shi et al. (2021) Strong selectivity and high capacity in the adsorption of As (V) from wastewater by glycine-modified Fe/Cu-layered double hydroxides https://doi.org/10.1016/j.jallcom.2021.158956
  60. Shi et al. (2021) Preparation of Mg, N-co-doped lignin adsorbents for enhanced selectivity and high adsorption capacity of As (V) from wastewater (pp. 206-213) https://doi.org/10.1016/j.partic.2021.03.014
  61. Kong et al. (2020) Enhanced removal of vanadium(V) from groundwater by layered double hydroxide-supported nanoscale zerovalent iron https://doi.org/10.1016/j.jhazmat.2020.122392
  62. Xue et al. (2022) Amorphous Mn-La oxides immobilized on carbon sphere for efficient removal of As(V), Cd(II), and Pb(II): Co-adsorption and roles of Mn species https://doi.org/10.1016/j.cej.2021.132262
  63. Threepanich and Praipipat (2021) Powdered and beaded lemon peels-doped iron (III) oxide-hydroxide materials for lead removal applications: Synthesis, characterizations, and lead adsorption studies 9(5) https://doi.org/10.1016/j.jece.2021.106007
  64. Tang et al. (2021) Phenylthiosemicarbazide-functionalized UiO-66-NH2 as highly efficient adsorbent for the selective removal of lead from aqueous solutions https://doi.org/10.1016/j.jhazmat.2021.125278
  65. Du et al. (2017) Highly efficient removal of Pb2+ by a polyoxomolybdate-based organic-inorganic hybrid material {(4-Hap)4[Mo8O26]} 5(2) (pp. 1866-1873) https://doi.org/10.1016/j.jece.2017.03.028
  66. Song et al. (2018) The selectively fluorescent sensing detection and adsorptive removal of Pb2+ with a stable [δ-Mo8O26]-based hybrid (pp. 598-604) https://doi.org/10.1016/j.jcis.2018.08.029
  67. Zhong et al. (2021) Design and syntheses of functionalized copper-based MOFs and its adsorption behavior for Pb(II) https://doi.org/10.1016/j.cclet.2021.1007.1040
  68. Yang et al. (2022) Functionalized dual modification of covalent organic framework for efficient and rapid trace heavy metals removal from drinking water https://doi.org/10.1016/j.chemosphere.2021.133215
  69. Morcos et al. (2021) High performance functionalized UiO metal organic frameworks for the efficient and selective adsorption of Pb (II) ions in concentrated multi-ion systems 9(3) https://doi.org/10.1016/j.jece.2021.105191
  70. Hong et al. (2022) Highly efficient removal of trace lead (II) from wastewater by 1,4-dicarboxybenzene modified Fe/Co metal organic nanosheets (pp. 212-218) https://doi.org/10.1016/j.jmst.2021.05.021
  71. Jing et al. (2022) Improving thermal conductivity of polyethylene/polypropylene by styrene-ethylene-propylene-styrene wrapping hexagonal boron nitride at the phase interface https://doi.org/10.1007/s42114-022-00438-x
  72. Wang et al. (2022) Broadband radar-absorbing performance of square-hole structure (pp. 525-535) https://doi.org/10.1007/s42114-021-00376-0
  73. Xin et al. (2021) Ultrahigh specific strength in a magnesium alloy strengthened by spinodal decomposition https://doi.org/10.1126/sciadv.abf3039
  74. Zhang et al. (2021) Correlation of C/C preform density and microstructure and mechanical properties of C/C-ZrC-based ultra-high-temperature ceramic matrix composites (pp. 743-750) https://doi.org/10.1007/s42114-021-00295-0
  75. Luo et al. (2021) Study on broadband microwave absorbing performance of gradient porous structure (pp. 591-601) https://doi.org/10.1007/s42114-021-00275-4
  76. Shao et al. (2021) Study on favorable comprehensive properties of superhydrophobic coating fabricated by polytetrafluoroethylene doped with graphene (pp. 521-533) https://doi.org/10.1007/s42114-021-00243-y
  77. Chen et al. (2021) Reinforced AZ91D magnesium alloy with thixomolding process facilitated dispersion of graphene nanoplatelets and enhanced interfacial interactions https://doi.org/10.1016/j.msea.2021.140793
  78. Zhao et al. (2019) Phase-field simulation for the evolution of solid/liquid interface front in directional solidification process
  79. Song et al. (2021) Waterborne polyurethane/3-amino-polyhedral oligomeric silsesquioxane (NH2-POSS) nanocomposites with enhanced properties (pp. 629-638) https://doi.org/10.1007/s42114-021-00285-2
  80. Chen et al. (2021) Three-dimensional phase-field simulations of the influence of diffusion interface width on dendritic growth of Fe-0.5 wt.%C alloy (pp. 371-378) https://doi.org/10.1007/s42114-021-00215-2
  81. Zhao et al. (2022) Fabrication of magnesium-coated graphene and its effect on the microstructure of reinforced AZ91 magnesium-matrix composites (pp. 504-512) https://doi.org/10.1007/s42114-021-00336-8
  82. Liu et al. (2020) Impact of lithium salts on the combustion characteristics of electrolyte under diverse pressures https://doi.org/10.3390/en13205373
  83. Lai et al. (2022) Aqueous flexible all-solid-state NiCo-Zn batteries with high capacity based on advanced ion-buffering reservoirs of NiCo2O4 https://doi.org/10.1007/s42114-021-00375-1
  84. Xu et al. (2022) Enhancement of catalytic combustion and thermolysis for treating polyethylene plastic waste https://doi.org/10.1007/s42114-021-00317-x
  85. Tan et al. (2022) Long-life and dendrite-free zinc metal anode enabled by a flexible, green and self-assembled zincophilic biomass engineered MXene based interface https://doi.org/10.1016/j.cej.2021.134277
  86. Liu et al. (2020) Phase change materials application in battery thermal management system: A review https://doi.org/10.3390/ma13204622
  87. Yu et al. (2022) Effect of pressure on anisotropy in elasticity, sound velocity, and thermal conductivity of vanadium borides https://doi.org/10.1007/s42114-021-00403-0
  88. Liu et al. (2021) Experimental thermal hazard investigation of pressure and EC/PC/EMC mass ratio on electrolyte 14(9) https://doi.org/10.3390/en14092511
  89. Zhao et al. (2022) Three-dimensional printing of the copper sulfate hybrid composites for supercapacitor electrodes with ultra-high areal and volumetric capacitances https://doi.org/10.1007/s42114-022-00430-5
  90. Shen et al. (2021) Nanoscale niobium oxides anode for electrochemical lithium and sodium storage: a review of recent improvements (pp. 33-68) https://doi.org/10.1007/s40097-020-00367-5
  91. Liu et al. (2021) High ion selectivity aquivion-based hybrid membranes for all vanadium redox flow battery (pp. 451-458) https://doi.org/10.1007/s42114-021-00261-w